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  1. We investigate the modes of deformation of an initially spherical bubble immersed in a homogeneous and isotropic turbulent background flow. We perform direct numerical simulations of the two-phase incompressible Navier–Stokes equations, considering a low-density bubble in the high-density turbulent flow at various Weber numbers (the ratio of turbulent and surface tension forces) using the air–water density ratio. We discuss a theoretical framework for the bubble deformation in a turbulent flow using a spherical harmonic decomposition. We propose, for each mode of bubble deformation, a forcing term given by the statistics of velocity and pressure fluctuations, evaluated on a sphere of the same radius. This approach formally relates the bubble deformation and the background turbulent velocity fluctuations, in the limit of small deformations. The growth of the total surface deformation and of each individual mode is computed from the direct numerical simulations using an appropriate Voronoi decomposition of the bubble surface. We show that two successive temporal regimes occur: the first regime corresponds to deformations driven only by inertial forces, with the interface deformation growing linearly in time, in agreement with the model predictions, whereas the second regime results from a balance between inertial forces and surface tension. The transition time between the two regimes is given by the period of the first Rayleigh mode of bubble oscillation. We discuss how our approach can be used to relate the bubble lifetime to the turbulence statistics and eventually show that at high Weber numbers, bubble lifetime can be deduced from the statistics of turbulent fluctuations at the bubble scale. 
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  2. We study bubble break-up in homogeneous and isotropic turbulence by direct numerical simulations of the two-phase incompressible Navier–Stokes equations. We create the turbulence by forcing in physical space and introduce the bubble once a statistically stationary state is reached. We perform a large ensemble of simulations to investigate the effect of the Weber number (the ratio of turbulent and surface tension forces) on bubble break-up dynamics and statistics, including the child bubble size distribution, and discuss the numerical requirements to obtain results independent of grid size. We characterize the critical Weber number below which no break-up occurs and the associated Hinze scale $d_h$ . At Weber number close to stable conditions (initial bubble sizes $d_0\approx d_h$ ), we observe binary and tertiary break-ups, leading to bubbles mostly between $0.5d_h$ and $d_h$ , a signature of a production process local in scale. For large Weber numbers ( $d_0> 3d_h$ ), we observe the creation of a wide range of bubble radii, with numerous child bubbles between $0.1d_h$ and $0.3d_h$ , an order of magnitude smaller than the parent bubble. The separation of scales between the parent and child bubble is a signature of a production process non-local in scale. The formation mechanism of these sub-Hinze scale bubbles relates to rapid large deformation and successive break-ups: the first break-up in a sequence leaves highly deformed bubbles which will break again, without recovering a spherical shape and creating an array of much smaller bubbles. We discuss the application of this scenario to the production of sub-Hinze bubbles under breaking waves. 
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  3. Although bubble pinch-off is an archetype of a dynamical system evolving toward a singularity, it has always been described in idealized theoretical and experimental conditions. Here, we consider bubble pinch-off in a turbulent flow representative of natural conditions in the presence of strong and random perturbations, combining laboratory experiments, numerical simulations, and theoretical modeling. We show that the turbulence sets the initial conditions for pinch-off, namely the initial bubble shape and flow field, but after the pinch-off starts, the turbulent time at the neck scale becomes much slower than the pinching dynamics: The turbulence freezes. We show that the average neck size, d ¯ , can be described by d ¯ ∼ ( t − t 0 ) α , where t 0 is the pinch-off or singularity time and α ≈ 0.5 , in close agreement with the axisymmetric theory with no initial flow. While frozen, the turbulence can influence the pinch-off through the initial conditions. Neck shape oscillations described by a quasi–2-dimensional (quasi-2D) linear perturbation model are observed as are persistent eccentricities of the neck, which are related to the complex flow field induced by the deformed bubble shape. When turbulent stresses are less able to be counteracted by surface tension, a 3-dimensional (3D) kink-like structure develops in the neck, causing d ¯ to escape its self-similar decrease. We identify the geometric controlling parameter that governs the appearance of these kink-like interfacial structures, which drive the collapse out of the self-similar route, governing both the likelihood of escaping the self-similar process and the time and length scale at which it occurs. 
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